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We have developed an approach based on ultrafast near-field microscopy that has allowed us to probe the nanoscale topography, crystallographic phase and chemical composition of metal halide perovskite films, while simultaneously extracting the ultrafast vertical carrier dynamics from femtosecond shifts in the pump-induced response following photoexcitation. This has revealed a surprising robustness of vertical charge transport towards nanoscale structural and compositional variations.
The results obtained in a close collaboration with the group of Michael Johnston (University of Oxford) have appeared in Nature Photonics.